Heterodyne gas cell measurements at 2.9 THz using a quantum cascade laser as local oscillator
(2010)
A terahertz (THz) heterodynespectrometer is demonstrated based on a quantum cascade laser(QCL) as a local oscillator (LO) and an NbN hot electron bolometer as a mixer, and it is used to measure high-resolution molecular spectral lines of methanol (CH 3 OH) between 2.913–2.918 THz. The spectral lines are taken from a gas cell containing methanol gas and using a single-mode QCL at 2.9156 THz as an LO, which is operated in the free running mode. By increasing the pressure of the gas, line broadening and saturation are observed. The measuredspectra showed good agreement with a theoretical model.
Superconducting heterodyne receiver has played a vital role in the high resolution spectroscopy applications for astronomy and atmospheric research up to 2THz. NbN hot electron bolometer (HEB) mixer, as the most sensitive mixer above 1.5THz, has been used in the Herschel space telescope for 1.4-1.9THz and has also shown an ultra-high sensitivity up to 5.3THz. Combined a HEB mixer with a novel THz quantum cascade laser (QCL) as local oscillator (LO), such an all solid-state heterodyne receiver provides the technology which can be used for any balloon-, air- and space-borne heterodyne instruments above 2THz. Here we report the first high-resolution heterodyne spectroscopy measurement using a gas cell and using such a HEB-QCL receiver. The receiver employs a 2.9THz metal-metal waveguide QCL as LO and a NbN HEB as a mixer. By using a gas cell filled with methanol (CH3OH) gas in combination with hot/cold blackbody loads as signal source, we successfully recorded the methanol emission line around 2.918THz. Spectral lines at different pressures and also different frequency of the QCL are studied.
A frequency tunable terahertz heterodynespectrometer, based on a third-order distributed feedback quantum cascade laser as a local oscillator, has been demonstrated by measuring molecular spectral lines of methanol (CH3OH) gas at 3.5 THz. By varying the bias voltage of the laser, we achieved a tuning range of ∼1 GHz of the lasing frequency, within which the molecular spectral lines were recorded. The measured spectra show excellent agreement with modeled ones. By fitting we derived the lasing frequency for each bias voltage accurately. The ultimate performance of the receiver including the resolution of noise temperature and frequency is also addressed.
