Prof. Dr. Stefanie Meilinger
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Departments, institutes and facilities
- Internationales Zentrum für Nachhaltige Entwicklung (IZNE) (57)
- Institut für Technik, Ressourcenschonung und Energieeffizienz (TREE) (56)
- Fachbereich Ingenieurwissenschaften und Kommunikation (54)
- Fachbereich Informatik (5)
- Fachbereich Wirtschaftswissenschaften (3)
- Institut für KI und Autonome Systeme (A2S) (1)
- Zentrum für Innovation und Entwicklung in der Lehre (ZIEL) (1)
Document Type
- Conference Object (34)
- Article (26)
- Report (5)
- Research Data (3)
- Preprint (3)
- Part of a Book (2)
- Contribution to a Periodical (2)
- Lecture (2)
- Working Paper (2)
- Diploma Thesis (1)
Year of publication
Keywords
- West Africa (6)
- energy meteorology (4)
- Global horizontal irradiance (3)
- AOD (2)
- COD (2)
- Distribution grid management (2)
- Energiemeteorologie (2)
- Erzeugungsprognose (2)
- Forecasting (2)
- Ghana (2)
For the winter 1999/2000 transport of air masses out of the vortex to mid-latitudes and ozone destruction inside and outside the northern polar vortex is studied to quantify the impact of earlier winter (before March) polar ozone destruction on mid-latitude ozone.
Nearly 112 000 trajectories are started on 1 December 1999 on 6 different potential temperature levels between 500–600 K and for a subset of these trajectories photo-chemical box-model calculations are performed. We linked a decline of −0.9% of mid-latitude ozone in this layer occurring in January and February 2000 to ozone destruction inside the vortex and successive transport of these air masses to mid-latitudes.
Further, the impact of denitrification, PSC-occurrence and anthropogenic chlorine loading on future stratospheric ozone is determined by applying various scenarios. Lower stratospheric temperatures and denitrification were found to play the most important role in the future evolution of polar ozone depletion.
Nitric acid partitioning in cirrus clouds: a synopsis based on field, laboratory and model studies
(2003)
From a synopsis of field, laboratory and model studies at T>205 K as well as from the field experiments POLSTAR at T<205 K we derive a general picture of the partitioning of nitric acid (HNO3) in cirrus clouds and a new hypothesis on the uptake of HNO3 on ice particles:
A substantial part of nitric acid remains in the gas phase under cirrus cloud conditions. The HNO3 removed from the gas phase is distributed between interstitial aerosol and ice particles in dependence on the temperature and ice surface, respectively. In cold cirrus clouds with small ice surface areas (T <205 K) the partitioning is strongly in favour of interstitial ternary solution particles while in warmer cirrus clouds with large ice surface areas the uptake on ice dominates. Consequently, denitrification via sedimenting ice particles may occur only in the -more frequently occurring- warm cirrus clouds
The HNO3 coverage on ice is found to be different for ice particles and ice films. On ice films the coverage can increase with decreasing temperature from about 0.1 to 0.8 monolayer, while that on ice particles is found to decrease with temperature and PHNO3 from 0.1 to 0.001 monolayer. An HNO3 uptake behaviour following dissociative Langmuir isotherms where the coverage decreases for descending temperatures may explain the observations for ice particles
From a comparison of the HNO3 measurements with model calculations it is found that (i) the global model of Lawrence and Crutzen (1998) overestimates the HNO3 partitioning in favour of the ice particles (ii) the Langmuir surface chemistry model of Tabazadeh et al. (1999) overestimates HNO3 coverages for temperatures ≤210 K More appropriate coverages are calculated when implementing in that model a temperature dependent function for the adsorption free energy (ΔGads (T)), which is empirically derived from the coverage measurements.
We examine the effect of nanometer-sized aircraft-induced aqueous sulfuric acid (H2SO4/H2O) particles on atmospheric ozone as a function of temperature. Our calculations are based on a previously derived parameterization for the regional-scale perturbations of the sulfate surface area density due to air traffic in the North Atlantic Flight Corridor (NAFC) and a chemical box model. We confirm large scale model results that at temperatures T>210 K additional ozone loss -- mainly caused by hydrolysis of BrONO2 and N2O5 -- scales in proportion with the aviation-produced increase of the background aerosol surface area. However, at lower temperatures (< 210 K) we isolate two effects which efficiently reduce the aircraft-induced perturbation: (1) background particles growth due to H2O and HNO3 uptake enhance scavenging losses of aviation-produced liquid particles and (2) the Kelvin effect efficiently limits chlorine activation on the small aircraft-induced droplets by reducing the solubility of chemically reacting species. These two effects lead to a substantial reduction of heterogeneous chemistry on aircraft-induced volatile aerosols under cold conditions. In contrast we find contrail ice particles to be potentially important for heterogeneous chlorine activation and reductions in ozone levels. These features have not been taken into consideration in previous global studies of the atmospheric impact of aviation. Therefore, to parameterize them in global chemistry and transport models, we propose the following parameterisation: scale the hydrolysis reactions by the aircraft-induced surface area increase, and neglect heterogeneous chlorine reactions on liquid plume particles but not on ice contrails and aircraft induced ice clouds.
This report has been prepared by the SETAC Europe Scientific Task Group on Global And RegionaL Impact Categories (SETAC-Europe/STG-GARLIC) that is installed by the 2nd SETAC Europe working group on life cycle impact assessment (WIA-2). This document is background to a chapter written by the same authors under the title “Climate change, stratospheric ozone depletion, photo-oxidant formation, acidification and eutrophication” in Udo de Haes et al. (2002). The chapter summarises the work of the STG-GARLIC and aims to give a state-of-the-art review of the best available practice(s) regarding category indicators and lists of concomitant characterisation factors for climate change, stratospheric ozone depletion, photo-oxidant formation, acidification, and aquatic and terrestrial eutrophication. Backgrounds on each of the specific impact categories are given in another background report from Klöpffer and Potting (2001).
This background report provides details on a selection of general issues relevant in relation to LCA and characterisation of impact in LCA. The document starts with a short introduction of the LCA methodology and impact assessment in LCA for non LCA-experts. LCA experts, on the other hand, will usually not be familiar in-depth with scientific and political backgrounds of the specific impact categories. A review of this is given. Also the discussion is provided about the issue of the position of the category indicator in the causality chain, and into the related issue of spatial differentiation. These two issues appeared to be one of the core items for SETAC-Europe/STG-GARLIC.
This thesis contributes to a better understanding of the effect of heterogeneous chemistry on ozone in the tropopause region. As part of the German research project ALTO, it especially focuses on the impact of aircraft emissions on heterogeneous ozone chemistry in this region. This is an important question as ozone is a strong greenhouse gas, whose radiative effect, is strongest near the tropopause.
In general, the treatment of heterogeneous processes on background and aviation-produced particles requires the consideration of processes ranging from nanometer to continental scale. For this reason the present modeling work includes a treatment of small scale processes as well as the development and subsequent application of parameterisations. Three numerical trajectory box models considering highly detailed microphysical and chemical processes have been developed: (a) an aircraft plume model including coagulation, chemistry and plume dilution, (b) a particle-size resolved microphysical box model and, (c) a comprehensive photo-chemical box model.
In this paper, a gas-to-power (GtoP) system for power outages is digitally modeled and experimentally developed. The design includes a solid-state hydrogen storage system composed of TiFeMn as a hydride forming alloy (6.7 kg of alloy in five tanks) and an air-cooled fuel cell (maximum power: 1.6 kW). The hydrogen storage system is charged under room temperature and 40 bar of hydrogen pressure, reaching about 110 g of hydrogen capacity. In an emergency use case of the system, hydrogen is supplied to the fuel cell, and the waste heat coming from the exhaust air of the fuel cell is used for the endothermic dehydrogenation reaction of the metal hydride. This GtoP system demonstrates fast, stable, and reliable responses, providing from 149 W to 596 W under different constant as well as dynamic conditions. A comprehensive and novel simulation approach based on a network model is also applied. The developed model is validated under static and dynamic power load scenarios, demonstrating excellent agreement with the experimental results.
The rapid increase in solar photovoltaic (PV) installations worldwide has resulted in the electricity grid becoming increasingly dependent on atmospheric conditions, thus requiring more accurate forecasts of incoming solar irradiance. In this context, measured data from PV systems are a valuable source of information about the optical properties of the atmosphere, in particular the cloud optical depth (COD). This work reports first results from an inversion algorithm developed to infer global, direct and diffuse irradiance as well as atmospheric optical properties from PV power measurements, with the goal of assimilating this information into numerical weather prediction (NWP) models.
In den Atmosphärenwissenschaften spielt die Strahlungsbilanz der Erde eine wichtige Rolle für unser Verständnis des Klimasystems. Hier liefern ausgereifte Satellitenprodukte dekadische Klimazeitreihen mit einer so hohen Genauigkeit, dass z.B. Änderungen im Zusammenhang mit dem Klimawandel detektiert werden können. Dies gilt insbesondere auch für die solaren Strahlungsflüsse an der Erdoberfläche. Beim Vergleich dieser Satellitenprodukte mit instantanen Beobachtungen der Strahlung am Erdboden sind jedoch oft erhebliche Abweichungen feststellbar, die hauptsächlich durch kleinskalige Variabilität in der räumlichen Struktur von Wolken und ihrer Strahlungswirkung verursacht werden. Hier ist auch zu bedenken, dass Bodenbeobachtungen fast einer Punktmessung entsprechen, während Satellitenpixel eine Fläche in der Größenordnung von Quadratkilometern abtasten.
West Africa has a great potential for the application of solar energy systems, as it combines high levels of solar irradiance with a lack of energy production. Southern West Africa is a region with a very high aerosol load. Urbanization, uncontrolled fires, traffic as well as power plants and oil rigs lead to increasing anthropogenic emissions. The naturally circulating north winds bring mineral dust from the Sahel and Sahara and monsoons - sea salt and other oceanic compounds from the south. The EU-funded Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa (DACCIWA) project (2014–2018), dlivered the most complete dataset of the atmosphere over the region to date. In our study, we use in-situ measured optical properties of aerosols from the airborne campaign over the Gulf of Guinea and inland, and from ground measurements in coastal cities.
In the research project "MetPVNet", both, the forecast-based operation management in distribution grids and as well as the forecasts of the feed-in of PV-power from decentralized plants could be improved on the basis of satellite data and numerical weather forecasts. Based on a detailed network analyses for a real medium-voltage grid area, it was shown that both – the integration of forecast data based on satellite and weather data and the improvement of subsequent day forecasts based on numerical weather models – have a significant added value for forecast-based congestion management or redispatch and reactive power management in the distribution grid. Furthermore, forecast improvements for the forecast model of the German Weather Service were achieved by assimilating visible satellite imagery, and cloud and radiation products from satellites were improved, thus improving the database for short-term forecasting as well as for assimilation. In addition, several methods have been developed that will enable forecast improvement in the future, especially for weather situations with high cloud induced variability and high forecast errors. This article summarizes the most important project results.
Anhand detaillierter Netzanalysen für ein reales Mittelspannungsnetzgebiet konnte gezeigt werden, dass sowohl die Einbindung von Prognosedaten auf Basis von Satelliten und Wetterdaten, als auch die Verbesserung von Folgetagsprognosen auf der Basis numerischer Wettermodelle einen deutlichen Mehrwert für ein prognosebasiertes Engpassmanagement bzw. Redispatch und Blindleistungsmanagement im Verteilnetz aufweisen. Auch Kurzfristprognosen auf der Basis von Satellitendaten haben einen positiven Effekt. Ein weiterer wichtiger Mehrwert des Projektes ist auch die Rückmeldung der kritischen Prognosesituationen aus Sicht der Anwendungsfälle, so dass wie bereits im Projekt gezeigt und darüber hinaus, Prognosen zielgerichteter auf die Anwendung im Verteilnetzbetrieb ausgelegt und optimiert werden können.
Weiterhin konnten Prognoseverbesserungen für das Vorhersagemodell des Deutschen Wetterdienstes durch die Assimilation von sichtbaren Satellitenbildern erreicht werden. Darüber hinaus wurden Wolken- und Strahlungsprodukte aus Satelliten verbessert und somit die Datenbasis für die Kurzfristprognose als auch für die Assimilation.
Darüber hinaus wurden verschiedene Methoden entwickelt, die zukünftig zu einer weiteren Prognoseverbesserung, insbesondere für Wettersituationen mit hohen Prognosefehlern, führen könnten. Solche Situationen wurden aus Sicht des Netzbetriebs und mithilfe von satellitenbasierten Analysen der Gesamtwetterlage für die Perioden der MetPVNet Messkampagnen identifiziert. Hierbei handelte es sich insbesondere um Situationen mit starker oder stark wechselhafter Bewölkung.
Für die MetPVNet Messkampagnen wurde auf der Basis eines Trainingsdatensatzes und in Abhängigkeit der Variabilitätsklasse die Abweichung der bodennahen Einstrahlung von Satellitendaten oder von Strahlungsprognosen quantifiziert. Diese Art der Informationen bietet zukünftig die Möglichkeit zur Bewertung der Prognosegüte.
The clear-sky radiative effect of aerosol–radiation interactions is of relevance for our understanding of the climate system. The influence of aerosol on the surface energy budget is of high interest for the renewable energy sector. In this study, the radiative effect is investigated in particular with respect to seasonal and regional variations for the region of Germany and the year 2015 at the surface and top of atmosphere using two complementary approaches.
First, an ensemble of clear-sky models which explicitly consider aerosols is utilized to retrieve the aerosol optical depth and the surface direct radiative effect of aerosols by means of a clear-sky fitting technique. For this, short-wave broadband irradiance measurements in the absence of clouds are used as a basis. A clear-sky detection algorithm is used to identify cloud-free observations. Considered are measurements of the short-wave broadband global and diffuse horizontal irradiance with shaded and unshaded pyranometers at 25 stations across Germany within the observational network of the German Weather Service (DWD). The clear-sky models used are the Modified MAC model (MMAC), the Meteorological Radiation Model (MRM) v6.1, the Meteorological–Statistical solar radiation model (METSTAT), the European Solar Radiation Atlas (ESRA), Heliosat-1, the Center for Environment and Man solar radiation model (CEM), and the simplified Solis model. The definition of aerosol and atmospheric characteristics of the models are examined in detail for their suitability for this approach.
Second, the radiative effect is estimated using explicit radiative transfer simulations with inputs on the meteorological state of the atmosphere, trace gases and aerosol from the Copernicus Atmosphere Monitoring Service (CAMS) reanalysis. The aerosol optical properties (aerosol optical depth, Ångström exponent, single scattering albedo and asymmetry parameter) are first evaluated with AERONET direct sun and inversion products. The largest inconsistency is found for the aerosol absorption, which is overestimated by about 0.03 or about 30 % by the CAMS reanalysis. Compared to the DWD observational network, the simulated global, direct and diffuse irradiances show reasonable agreement within the measurement uncertainty. The radiative kernel method is used to estimate the resulting uncertainty and bias of the simulated direct radiative effect. The uncertainty is estimated to −1.5 ± 7.7 and 0.6 ± 3.5 W m−2 at the surface and top of atmosphere, respectively, while the annual-mean biases at the surface, top of atmosphere and total atmosphere are −10.6, −6.5 and 4.1 W m−2, respectively.
The retrieval of the aerosol radiative effect with the clear-sky models shows a high level of agreement with the radiative transfer simulations, with an RMSE of 5.8 W m−2 and a correlation of 0.75. The annual mean of the REari at the surface for the 25 DWD stations shows a value of −12.8 ± 5 W m−2 as the average over the clear-sky models, compared to −11 W m−2 from the radiative transfer simulations. Since all models assume a fixed aerosol characterization, the annual cycle of the aerosol radiation effect cannot be reproduced. Out of this set of clear-sky models, the largest level of agreement is shown by the ESRA and MRM v6.1 models.
Background & Objective: Due to the policy goals for sustainable energy production, renewable energy plants such as photovoltaics are increasingly in use. The energy production from solar radiation depends strongly on atmospheric conditions. As the weather mostly changes, electrical power generation fluctuates, making technical planning and control of power grids to a complex problem. Due to used materials (semiconductors e.g. silicon, gallium arsenide, cadmium telluride) the photovoltaic cells are spectrally selective. It means that only radiation of certain wavelengths converts into electrical energy. A material property called spectral response characterizes a certain degree of conversion of solar radiation into the electric current for each wavelength of solar light.